Bring 2/3 cup water and sugar to boil in medium saucepan, stirring until sugar dissolves.
Remove from heat; cool syrup completely. Puree 2 cups raspberries in processor.
Pour puree through fine strainer set over saucepan with syrup. Press on solids to extract as much liquid as possible; discard solids.
Mix orange juice, next 6 ingredients, 1 cup berries, and raspberry syrup in glass bowl. Cover; chill at least 4 hours and up to 1 day. Strain into pitcher.