Cut bread loaf into 8 (1-inch-thick) slices; cut slices in half, if desired.
Drizzle tomatoes and onion with 2 Tbsp. oil, tossing to coat.
Grill tomatoes and onion, covered with grill lid, over 350 to 400 (medium-high) heat 3 to 4 minutes on each side or until lightly charred.
Coarsely chop grilled tomatoes and onion, and place in a medium bowl.
Add 2 Tbsp. oil, cucumber, and next 3 ingredients. Season with salt and pepper to taste.
Brush bread slices with remaining 1 Tbsp. olive oil. Grill, without grill lid, over 350 to 400 (medium-high) heat 1 to 2 minutes on each side or until lightly browned and toasted.
Place grilled bread slices on individual serving plates; top with tomato mixture.